Search for dissertations about: "excited state dipole moment"

Showing result 1 - 5 of 11 swedish dissertations containing the words excited state dipole moment.

  1. 1. Light Control using Organometallic Chromophores

    Author : Johan Henriksson; Patrick Norman; Olav Vahtras; Linköpings universitet; []
    Keywords : NATURVETENSKAP; NATURAL SCIENCES; organometallic chromophores; two-photon absorption; excited state absorption; excited state dipole moment; four-component formalism; clamping levels; spin-transition; Computational physics; Beräkningsfysik;

    Abstract : The interaction between light and organometallic chromophores has been investigated theoretically in a strive for fast optical filters. The main emphasis is on two-photon absorption and excited state absorption as illustrated in the Jablonski diagram. We stress the need for relativistic calculations and have developed methods to address this issue. READ MORE

  2. 2. Stark Spectroscopy, Lifetimes and Coherence Effects in Diatomic Molecular Systems

    Author : Annie Hansson; Peder Royen; Michel Herman; Stockholms universitet; []
    Keywords : NATURVETENSKAP; NATURAL SCIENCES; diatomic; dipole moment; Stark effect; lifetimes; transition moment; coherence effects; EIT; Autler-Townes; Chemical physics; Kemisk fysik;

    Abstract : In this dissertation is exemplified how different laser based methods are applied in high-resolution spectroscopic studies of internal properties of diatomic molecules.A molecular beam apparatus assembly is described, where a laser ablation source is combined with a time-of-flight mass spectrometer. READ MORE

  3. 3. Cerium as a quantum state probe for rare-earth qubits in a crystal

    Author : Jenny Karlsson; Atomfysik; []
    Keywords : NATURVETENSKAP; NATURAL SCIENCES; Spectroscopy; Quantum Computing; Rare-earth-ion-doped crystals; Microscopy; Fysicumarkivet A:2015:Karlsson;

    Abstract : Rare-earth ions doped into a transparent crystal can have optically excited states with coherence times of milliseconds and hyperfine levels with coherence times of hours when cooled down to liquid helium temperatures. This makes them attractive for developing quantum computing hardware. READ MORE

  4. 4. Ultrafast Photo-induced Reaction Dynamics of Small Molecules

    Author : Malin Kadi; Jan Davidsson; Eva Åkesson; Sören Keiding; Uppsala universitet; []
    Keywords : NATURVETENSKAP; NATURAL SCIENCES; Physical chemistry; pump-probe spectroscopy; reaction dynamics; photodissociation; aryl halides; spin-orbit coupling; ab initio calculations; molecular dynamics; vibrational wavepackets; Fysikalisk kemi; Physical chemistry; Fysikalisk kemi;

    Abstract : The main focus of this thesis is the investigation of the dissociation dynamics of aryl halides using femtosecond pump-probe spectroscopy. In the monohalogenated aryl halides, iodo-, bromo- and chlorobenzene, the rate of dissociation following excitation at 266 nm in the gas phase increased with increasing mass of the halogen atom. READ MORE

  5. 5. Towards single Ce ion detection in a bulk crystal for the development of a single-ion qubit readout scheme

    Author : Ying Yan; Atomfysik; []
    Keywords : NATURVETENSKAP; NATURAL SCIENCES; Fysicumarkivet A:2013:Yan; Ultra-violet laser spectroscopy; Single ion detection; Rare-earth-ion-doped crystals; Quantum computing; Laser stabilisation;

    Abstract : The work presented in this thesis was concerned with investigating the relevant spectroscopic properties of Ce ions randomly doped in an Y2SiO5 crystal at low temperatures (around 4 K), in order to develop a technique and an experimental set-up to detect the fluorescence photons emitted by a single Ce ion. The aim of the work was to determine whether a single Ce ion (referred to as the readout ion) can be used as a local probe to sense the quantum state of a neighbouring single-ion qubit via a state-selective interaction between the readout and qubit ion. READ MORE